Semiclassical Nonadiabatic Dynamics Based on Quantum Trajectories for the O(3P,1D) + H2 System

Sophya V. Garashchuk, University of South Carolina - Columbia
V. A. Rassolov
G. C. Schatz

Copyright 2006 American Institute of Physics. This article may be downloaded for personal use only. Any other use requires prior permission of the author and the American Institute of Physics.

The following article appeared in

Garashchuk, S., Rassolov, V. A., & Schatz, G. C. (2006). Semiclassical nonadiabatic dynamics based on quantum trajectories for the O(3P,1D) + H2 system. The Journal of Chemical Physics, 124, 244307. http://dx.doi.org/10.1063/1.2208615

and may be found at

http://scitation.aip.org/content/aip/journal/jcp/124/24/10.1063/1.2208615

Abstract

The O(P3,D1)+H2→OH+Hreaction is studied using trajectory dynamics within the approximate quantum potential approach. Calculations of the wave-packet reaction probabilities are performed for four coupled electronic states for total angular momentum J=0 using a mixed coordinate/polar representation of the wave function. Semiclassical dynamics is based on a single set of trajectories evolving on an effective potential-energy surface and in the presence of the approximate quantum potential. Population functions associated with each trajectory are computed for each electronic state. The effective surface is a linear combination of the electronic states with the contributions of individual components defined by their time-dependent average populations. The wave-packet reaction probabilities are in good agreement with the quantum-mechanical results. Intersystem crossing is found to have negligible effect on reaction probabilities summed over final electronic states.