High Performance Low Temperature Solid Oxide Fuel Cells with Novel Electrode Architecture

Author(s)

Yu Chen
Qian Liu
Zhibin Yang
Fanglin Chen, University of South Carolina - ColumbiaFollow
Minfang Han

Document Type

Article

Abstract

In this study, we have fabricated high performance low temperature solid oxide fuel cells (LT-SOFCs) with both acicular anodes and cathodes with thin Gd-doped ceria (GDC) electrolyte film. The acicular Ni-Gd_0.1Ce_0.9O_2−δ (Ni-GDC) anode was prepared using freeze drying tape casting, while the hierarchically porous cathode with nano-size Sm_0.5Sr_0.5CoO₃ (SSC) particles covering an acicular GDC skeleton was prepared by a combination of freeze drying tape casting and self-rising approaches. The acicular electrodes with 5–200 μm pores/channels enhance mass transport, while SSC particles of about 50 nm in the cathode promote electrochemical reactions. Cells which have this novel electrode architecture show a significantly high power output of 1.44 W cm⁻² and an extremely low cell polarization resistance of 0.0379 Ω cm² at 600 °C.

Publication Info

Published in RSC Advances, Volume 21, Issue 32, 2012, pages 12118-12121.

©RSC Advances 2012, Royal Society of Chemistry.

This article cannot be redistributed or further made available. This article was first published by the Royal Society of Chemistry and can be found at http://dx.doi.org/10.1039/C2RA21921B

Chen, Y., Liu, Q., Yang, Z., Chen, F. & Han, M. (14 December 2012). High Performance Low Temperature Solid Oxide Fuel Cells with Novel Electrode Architecture. RSC Advances, 2 (32), 12118 – 12121. http://dx.doi.org/10.1039/C2RA21921B

Rights

©RSC Advances 2012, Royal Society of Chemistry.

This article cannot be redistributed or further made available. This article was first published by the Royal Society of Chemistry and can be found at http://dx.doi.org/10.1039/C2RA21921B

Chen, Y., Liu, Q., Yang, Z., Chen, F. & Han, M. (14 December 2012). High Performance Low Temperature Solid Oxide Fuel Cells with Novel Electrode Architecture. RSC Advances, 2 (32), 12118 – 12121. http://dx.doi.org/10.1039/C2RA21921B